Summary
Sorption-induced strain and permeability were measured as a function of pore
pressure using subbituminous coal from the Powder River basin of Wyoming, USA,
and high-volatile bituminous coal from the Uinta-Piceance basin of Utah, USA.
We found that for these coal samples, cleat compressibility was not constant,
but variable. Calculated variable cleat-compressibility constants were found to
correlate well with previously published data for other coals. Sorption-induced
matrix strain (shrinkage/swelling) was measured on unconstrained samples for
different gases: carbon dioxide (CO2), methane (CH4), and
nitrogen (N2). During permeability tests, sorption-induced matrix
shrinkage was demonstrated clearly by higher-permeability values at lower pore
pressures while holding overburden pressure constant; this effect was more
pronounced when gases with higher adsorption isotherms such as CO2
were used. Measured permeability data were modeled using three different
permeability models that take into account sorption-induced matrix strain. We
found that when the measured strain data were applied, all three models matched
the measured permeability results poorly. However, by applying an
experimentally derived expression to the strain data that accounts for the
constraining stress of overburden pressure, pore pressure, coal type, and gas
type, two of the models were greatly improved.
Introduction
Coal seams have the capacity to adsorb large amounts of gases because of
their typically large internal surface area (30 to 300 m2/g)
(Berkowitz 1985). Some gases, such as CO2, have a higher affinity
for the coal surfaces than others, such as N2. Knowledge of how the
adsorption or desorption of gases affects coal permeability is important not
only to operations involving the production of natural gas from coalbeds but
also to the design and operation of projects to sequester greenhouse gases in
coalbeds (RECOPOL Workshop 2005).
As reservoir pressure is lowered, gas molecules are desorbed from the matrix
and travel to the cleat (natural-fracture) system, where they are conveyed to
producing wells. Fluid movement in coal is controlled by diffusion in the coal
matrix and described by Darcy flow in the fracture (cleat) system. Because
diffusion of gases through the matrix is a much slower process than Darcy flow
through the fracture (cleat) system, coal seams are treated as fractured
reservoirs with respect to fluid flow. However, coalbeds are more complex than
other fractured reservoirs because of their ability to adsorb (or desorb) large
quantities of gas.
Adsorption of gases by the internal surfaces of coal causes the coal matrix
to swell, and desorption of gases causes the coal matrix to shrink. The
swelling or shrinkage of coal as gas is adsorbed or desorbed is referred to as
sorption-induced strain. Sorption-induced strain of the coal matrix causes a
change in the width of the cleats or fractures that must be accounted for when
modeling permeability changes in the system. A number of permeability-change
models (Gray 1987; Sawyer et al.
1990; Seidle and Huitt 1995; Palmer and Mansoori 1998; Pekot and Reeves 2003;
Shi and Durucan 2003) for coal have been proposed that attempt to account
for the effect of sorption-induced strain. Accurate measurement of
sorption-induced strain becomes important when modeling the effect of gas
sorption on coal permeability.
For this work, laboratory measurements of sorption-induced strain were made
for two different coals and three gases. Permeability measurements also were
made using the same coals and gases under different pressure and stress
regimes. The objective of this current work is to present these data and to
model the laboratory-generated permeability data using a number of
permeability-change models that have been described by other researchers. This
work should be of value to those who model coalbed-methane fields with
reservoir simulators because these results could be incorporated into those
reservoir models to improve their accuracy.
© 2007. Society of Petroleum Engineers
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